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Structural, Electronic and Magnetic Properties of Spinel Based Transition Metal Oxides

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Author

Khan, Mahmood

Program

PhD

Institute

Hazara University

City

Mansehra

Province

KPK

Country

Pakistan

Thesis Completing Year

2018

Thesis Completion Status

Completed

Subject

Physics

Language

English

Link

http://prr.hec.gov.pk/jspui/bitstream/123456789/12645/1/Mahmood%20Khan_Phy_2018_Hazara_PRR.pdf

Added

2021-02-17 19:49:13

Modified

2024-03-24 20:25:49

ARI ID

1676727248295

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Theoretical study of Spinel based Transition Metal Oxides is reported. The Density Functional Theory approach is adopted for computational investigation using LAPW code. The structural, elastic properties of (XAl2O4 for X=Mg, Mn, Fe, Co, Ni, Cu, Zn), (MGa2O4 for M=Mg, Mn, Fe, Co, Ni, Cu, Zn, Cd), (NIn2O4 for N=Mg, Zn, In) & (ZnP2O4 for P=V, Cr, Fe, Rh, Sn) along with electronic & magnetic properties of cubic spinel oxides (XAl2O4) and (MGa2O4) have calculated. The calculated structural parameters conform to other experimental and theoretical evidences. Fulfillment of elastic stability criteria proves the reliability of the reported data. The calculated elastic constants show that all materials abide its stability opposing elastic deformations and the Cauchy’s pressure confirms the dynamical stability of these materials. The high values of bulk moduli show the hardness of these materials while the Young moduli data reveal that MgAl2O4 is the stiffer material among all. Further, Poisson’s ratios testify the compressibility, connote stableness to external deformation of these materials and reveal dominance of central forces being the interatomic forces. Out of 24 materials, only 05 are brittle and the rest are ductile with elastic anisotropy. MgAl2O4 is the most brittle and CdGa2O4 is the most ductile material. The electronic structure (Total DOS) show all XAl2O4, MGa2O4 (M=Fe, Co, Zn, Cd) have antiferromagnetic, NiGa2O4 & CuGa2O4 have FM state and the valence near Fermi level due to the transition metal 3d state. The calculation of direct exchange energy Δx(d) shows that the exchange mechanism of electrons is dominant in introducing magnetism and enormous exchange splitting is observed in these materials. The ferromagnetism in the group MGa2O4 of spinel oxide compounds is due to hybridization between the electrons in the 3d-states cation and 2p states anion. Appearance of magnetic moments in these materials is due to unpaired electrons in 3d states of Transition metal ions. The negative value of indirect exchange energy confirms the magnetism by spin of electrons.
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ملن دی چاہ

ملن دی چاہ
بس نوں ٹور ڈریورا میں ملنا ہے دلدار
جہلم جا روک لویں میں تکنا سوہنا یار

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ڈھونڈ تھکی میں ہر اک پاسا
لبھدی پھراں میں پھڑ کے کاسا
میں اپڑی جہلم بازار

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ویکھن والیاں دے دل موہندے
نین تے ہنجواں ہار پروندے
سوہنا ملسی کیہڑے وار

میں ٹلے تے آن کھلوواں
سد ماراں تے نالے روواں
کر کر توبہ اگلے دھوواں
رب چا بخشے اوگنہار

جہلم پل توں ٹلا دِسے
جتھے سجناں تے دل وِسے
قادریؔ عشق دے لمے قصے
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ٹلا جوگیاں من نوں بھاوے
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